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31. 32. 33. 34. 35. 36. 37. 38. 39. 40. 41. 42. 43. 44. 45. 46. 47. 41 LA,Vega C,Viguri F (1997) Chem Commun 2351; (j) Hollis TK, Odenkirk W, Robinson NP, Whelan J, Bosnich B (1993) Tetrahedron 49:5415; (k) Odenkirk W, Rheingold AL, Bosnich B (1992) J Am Chem Soc 114:6392 Kündig EP, Saudan CM, Alezra V, Viton F, Bernardinelli G (2001) Angew Chem Int Ed Engl 40:4481 Faller JW, Grimmond BJ, D’Alliessi DG (2001) J Am Chem Soc 123:2525 Viton F, Bernardinelli G, Kündig EP (2002) J Am Chem Soc 124:4968 Ellis WW, Odenkirk W, Bosnich B (1998) Chem Commun 1311 Sato S, Matsuda I, Shibata M (1989) J Organomet Chem 377:347 (a) Itoh K, Masuda K, Fukahori T, Nakano K, Aoki K, Nagashima H (1994) Organometallics 13:1020; (b) Masuda K, Nakano K, Fukahori T, Nagashima H, Itoh K (1992) J Organomet Chem 428:C21 (a) Trost BM, Pinkerton AB, Seidel M (2001) J Am Chem Soc 123:12466; (b) Trost BM, Pinkerton AB (1999) J Am Chem Soc 121:4068 Trost BM, Pinkerton AB (1999) J Am Chem Soc 121:10842 Trost BM, Pinkerton AB, Kremzow D (2000) J Am Chem Soc 122:12007 Yoshida M, Sugimoto K, Ihara M (2001) Tetrahedron Lett 42:3877 Kang S-K, Ko B-S, Lee D-M (2002) Tetrahedron Lett 43:6693 Mitsudo T-a, Zhang S-W, Nagao M, Watanabe Y(1991) J Chem Soc Chem Commun 598 (a) Trost BM, Chisholm JD, Wrobleski ST, Jung M (2002) J Am Chem Soc 124:12420; (b) Lopez F, Castedo L, Mascarenas JL (2002) J Am Chem Soc 124:4218; (c) Trost BM, Shen HC, Pinkerton AB (2002) Chem Eur J 8:2341; (d) Trost BM, Toste FD (1999) Tetrahedron Lett 40:7739; (e) Trost BM, Roth GJ (1999) Org Lett 1:67; (f) Trost BM, Probst GD, Schoop A (1998) J Am Chem Soc 120:9228; (g) Trost BM, Indolese A (1993) J Am Chem Soc 115:4361 Trost BM, Indolese AF, Müller TJJ, Treptow B (1995) J Am Chem Soc 117:615 Trost BM, Pinkerton AB, Toste FD, Sperrle M (2001) J Am Chem Soc 123:12504 (a) Trost BM, Calkins TL, Bochet CG (1997) Angew Chem Int Ed Engl 36:2632; (b) Trost BM, Müller TJJ, Martinez J (1995) J Am Chem Soc 117:1888; (c) Trost BM, Calkins TL (1995) Tetrahedron Lett 36:6021; (d) Trost BM, Müller TJJ (1994) J Am Chem Soc 116:4985 (a) Trost BM, Machacek MR, Ball ZT (2003) Org Lett 5:1895; (b) Trost BM, Machacek MR (2002) Angew Chem Int Ed Engl 41:4693; (c) Trost BM, Machacek MR, Schnaderbeck MJ (2000) Org Lett 2:1761 Trost BM, Martinez JA, Kulawiec RJ, Indolese AF (1993) J Am Chem Soc 115:10402 (a) Trost BM, Surivet J-P (2001) Angew Chem Int Ed Engl 40:1468; (b) Trost BM, Surivet J-P, Toste FD (2001) J Am Chem Soc 123:2897 (a) Dérien S, Jan D, Dixneuf P-H (1996) Tetrahedron 52:5511; (b) Dérien S, Dixneuf P-H (1994) J Chem Soc Chem Commun 2551 (a) Dérien S, Ropartz L, Le Paih J, Dixneuf P-H (1999) J Org Chem 64:3524; (b) Dérien S, Gomez Vicente B, Dixneuf P-H (1997) Chem Commun 1405 Yi CS, Lee DW, Chen Y (1999) Organometallics 18:2043 Kakiuchi F, Uetsuhara T, Tanaka Y, Chatani N, Murai S (2002) J Mol Catal A 182–183: 511 Mitsudo T-a, Naruse H, Kondo T, Ozaki Y, Watanabe Y (1994) Angew Chem Int Ed Engl 33:580 Mitsudo T-a, Kokuryo K, Shinsugi T, Nakagawa Y,Watanabe Y, Takegami Y (1979) J Org Chem 44:4492 (a) Jordan RW, Tam W (2002) Tetrahedron Lett 43:6051; (b) Jordan RW, Tam W (2001) Org Lett 3:2367; (c) Jordan RW, Tam W (2000) Org Lett 2:3031 42 S.

2 Addition to Acetylenes . . . . . . . . . . . . . . . . 65 65 67 . . . . . . . . 68 4 Reaction of Aldehydes and Related Compounds 5 Reaction of Active Methylene and Related Compounds . . . . . . 72 6 Conclusion . . . . . . . . . . . . . . . . . . . 76 References . . . . . . . . . . . . . . . . . . . . 76 Abstract The development of catalytic reactions involving carbon–hydrogen bond cleavage is one of the most attractive research subjects in organic and organometallic chemistries.

The introduction of an optically pure chelating cyclopentadienylphosphine ligand with planar chirality leads to the creation of the new C–C bond with very high enantioselectivity from symmetrical carbonates and sodiomalonates [113]. (85) The observation that the Ru(amidinate)C5Me5 complex could generate the first allyl ruthenium(IV) complex containing a nitrogen ligand led to the use of this complex as catalyst for simple allyl substitution of allylcarbonates [111]. Re- 36 S. Dérien et al. cently, it has been shown that Cp*Ru(bisimine)Cl also catalyzes the nucleophilic substitution of allylic carbonates [114] and that [Cp*Ru(bipyridine)(MeCN)]PF6 catalysts provide a highly regioselective nucleophilic substitution with C, N, and O nucleophiles via a dicationic ruthenium(IV) intermediate without previous deprotonation of the carbonucleophile precursor [115].

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